Product Details of 100-51-6. Kang, XC; Lyu, K; Li, LL; Li, JN; Kimberley, L; Wang, B; Liu, LF; Cheng, YQ; Frogley, MD; Rudic, S; Ramirez-Cuesta, AJ; Dryfe, RAW; Han, BX; Yang, SH; Schroder, M in [Kang, Xinchen; Lyu, Kai; Li, Lili; Li, Jiangnan; Kimberley, Louis; Wang, Bin; Dryfe, Robert A. W.; Yang, Sihai; Schroder, Martin] Univ Manchester, Sch Chem, Manchester M13 9PL, Lancs, England; [Liu, Lifei; Han, Buxing] Chinese Acad Sci, Beijing Natl Lab Mol Sci, Key Lab Colloid Interface & Chem Thermodynam, Inst Chem, Beijing 100190, Peoples R China; [Cheng, Yongqiang; Ramirez-Cuesta, Anibal J.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA; [Frogley, Mark D.] Diamond Light Source, Harwell Sci Campus, Didcot OX11 0DE, Oxon, England; [Rudic, Svemir] STFC Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England published Integration of mesopores and crystal defects in metal-organic frameworks via templated electrosynthesis in 2019.0, Cited 45.0. The Name is Benzyl Alcohol. Through research, I have a further understanding and discovery of 100-51-6.
Incorporation of mesopores and active sites into metal-organic framework (MOF) materials to uncover new efficient catalysts is a highly desirable but challenging task. We report the first example of a mesoporous MOF obtained by templated electrosynthesis using an ionic liquid as both electrolyte and template. The mesoporous Cu(II)-MOF MFM-100 has been synthesised in 100 seconds at room temperature, and this material incorporates crystal defects with uncoupled Cu(II) centres as evidenced by confocal fluorescence microscopy and electron paramagnetic resonance spectroscopy. MFM-100 prepared in this way shows exceptional catalytic activity for the aerobic oxidation of alcohols to produce aldehydes in near quantitative yield and selectivity under mild conditions, as well as having excellent stability and reusability over repeated cycles. The catalyst-substrate binding interactions have been probed by inelastic neutron scattering. This study offers a simple strategy to create mesopores and active sites simultaneously via electrochemical formation of crystal defects to promote efficient catalysis using MOFs.
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Reference:
Indole alkaloid derivatives as building blocks of natural products from Bacillus thuringiensis and Bacillus velezensis and their antibacterial and antifungal activity study,
,Preparation of Indole Containing Building Blocks for the Regiospecific Construction of Indole Appended Pyrazoles and Pyrroles